Background: Diffuse midline gliomas (DMG), including those located in the brainstem (diffuse intrinsic pontine glioma – DIPG) comprise almost half of all paediatric high grade gliomas and are considered the most lethal of all children’s cancers. DIPG harbours a median overall survival of 9-11-months, where the only approved treatment is palliative radiotherapy. Preliminary clinical efficacy for the small molecule brain-penetrant drug ONC201 shows an emerging survival benefit in early-stage clinical trials (NCT03416530), however, many patients do not respond, and all patients become resistant.
Aim: To uncover the mechanisms by which DIPG cell lines escape cell death following ONC201 treatment, and use these data to design strategies to improve response.
Methods: Initial testing revealed 10/13 patient-derived DIPG cell lines responded to ONC201. To uncover mechanisms of resistance, we performed quantitative proteomics on the H3.3K27M TP53-mutant ONC201 resistant line, SU-DIPG-VI, +/-ONC201 grown under hypoxic and normoxic conditions.
Results: Pathway analysis of proteomic profiling results identified mitochondrial degradation as the most enriched biological process. ONC201 is known to be a potent agonist of the mitochondrial protease CLPP, hence proteolysis and degradation of electron transport chain proteins including SDHA, and TCA cycle proteins including IDH3, were seen following 24 h treatment. The loss of mitochondrial integrity, including TCA cycle activity, promoted metabolic alterations to the epigenome, including increased trimethylation of H3K4 and H3K27. Therapeutic rescue was underpinned by redox-activated PI3K/AKT signalling, prompting the use of the blood-brain barrier permeable, clinically relevant PI3K/AKT inhibitor, paxalisib (NCT0396355). The combination with ONC201 was synergistically cytotoxic in both ONC201 sensitive and resistant DIPG cell lines, however, not in normal control peripheral blood mononuclear cells. Synergism was also seen in vivo using the SU-DIPG-VI-patient derived xenograft mouse model (p=0.0043). This combination was provided under compassionate access for two DIPG patients. Case 1, 6-year-old DIPG patient 6-weeks post-radiotherapy received the combination of ONC201 (15 mg/kg weekly) and paxalisib (27mg/m2 daily). Patient continues to receive the combination, 15-months after diagnosis and has experienced an almost complete regression of the primary tumour. Case 2, 16-year-old DIPG patient, commenced the combination following re-irradiation, 18-months post-diagnosis. Patient experienced a 34% reduction in tumour volume, with marked resolution of neurological symptoms, but unfortunately passed away from pneumocystis pneumonia 23-months after diagnosis.
Conclusions: Our preclinical and case study results underpin the recently commenced phase II clinical trial (NCT05009992), testing the combination of ONC201 and paxalisib immediately post-radiotherapy, or for patients in disease progression, immediately post re-irradiation.